Title

Novel Synthesis of Divergent Aryl Imidazoles from Ketones Involving Copper-Catalyzed α-amination and Oxidative C-C Bond Cleavage

Funding Source

Higher Education Discipline Innovation Project, Sichuan University, National Natural Science Foundation of China

Grant Number

B18035, 2017 CDLZ-S34, 21072131

Department

Department of Chemistry

Document Type

Article

Publication Date

4-6-2020

Abstract

A one-pot synthesis, initiated by a copper salt with inorganic (NH4)2CO3 as the nitrogen source, forms divergent aryl imidazole derivatives from ketones via a-amination and oxidative C–C bond cleavage reactions. The approach provides a simple and rapid synthesis of imidazole derivatives and has certain versatility.

Comments

DOI: 10.1039/d0ra01408g

Funding text

We gratefully acknowledge the nancial support from the National Natural Science Foundation of China (No. 21072131), 111 project (B18035) and Sichuan University – Lu Zhou Strategic Cooperation Projects (No. 2017 CDLZ-S34).

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